USB 3 is the simplest method that allows for a fast connection, just make sure you use an USB3 port on the PC. Alternatively, you'd need to have a Gigabit Ethernet set, with both your PC having a Gigabit Network adapter, and going through a gigabit switch to the NAS, with Cat-6 cables. The Gigabit LAN setup would allow multiple PCs to connect/use the NAS at the higher speeds, typically around 80 Megabytes/sec. Not sure what your router LAN-side switch speed is, and how your PC is connected to it.
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